Tom Cruise was originally cast as Napoleon Solo in Operazione U.N.C.L.E. (2015) before being forced to drop out as the production for the previous installment, Mission: Impossible - Rogue Nation (2015), clashed with Operazione U.N.C.L.E. (2015). As a result, Henry Cavill was moved up to play Napoleon. Impressed by his replacement and wanting to work with Cavill, he proposed to Christopher McQuarrie to cast him as Agent Walker. It was also Cruise's idea to have Vanessa Kirby cast as The White Widow since Cruise was impressed by her work as Princess Margaret in the first two seasons of The Crown (2016).

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